High-performance inorganic metal halide perovskite transistors
نویسندگان
چکیده
Abstract The p-type characteristic of solution-processed metal halide perovskite transistors means that they could be used in combination with their n-type counterparts, such as indium–gallium–zinc-oxide transistors, to create complementary metal–oxide–semiconductor-like circuits. However, the performance and stability perovskite-based do not yet match which limit broader application. Here we report high-performance p-channel thin-film based on inorganic caesium tin triiodide semiconducting layers have moderate hole concentrations high Hall mobilities. channels are formed by engineering film composition crystallization process using a tin-fluoride-modified caesium-iodide-rich precursor lead substitution. optimized exhibit field-effect mobilities over 50 cm 2 V ?1 s on/off current ratios exceeding 10 8 , well operational reproducibility.
منابع مشابه
Metal halide perovskite light emitters.
Twenty years after layer-type metal halide perovskites were successfully developed, 3D metal halide perovskites (shortly, perovskites) were recently rediscovered and are attracting multidisciplinary interest from physicists, chemists, and material engineers. Perovskites have a crystal structure composed of five atoms per unit cell (ABX3) with cation A positioned at a corner, metal cation B at t...
متن کاملIonic behavior of organic-inorganic metal halide perovskite based metal-oxide-semiconductor capacitors.
Organic-inorganic metal halide perovskites are promising semiconductors for optoelectronic applications. Despite the achievements in device performance, the electrical properties of perovskites have stagnated. Ion migration is speculated to be the main contributing factor for the many unusual electrical phenomena in perovskite-based devices. Here, to understand the intrinsic electrical behavior...
متن کاملMetal halide perovskite nanomaterials: synthesis and applications
Nanomaterials refer to those with at least one dimension being at the nanoscale (i.e. <100 nm) such as quantum dots, nanowires, and nanoplatelets. These types of materials normally exhibit optical and electrical properties distinct from their bulk counterparts due to quantum confinement or strong anisotropy. In this perspective, we will focus on a particular material family: metal halide perovs...
متن کاملAll-inorganic cesium lead halide perovskite nanocrystals for photodetector applications.
Herein, we describe simple, fast and reproducible halide ion exchange reactions in CsPbX3 (X = Cl, Br, I) nanocrystals (NCs) at room temperature. Through the simple adjustment of the halide ion concentration, the photoluminescence of these NCs can be tuned over the entire visible region (425-655 nm). Photodetector devices based on entirely inorganic CsPbI3 NCs are demonstrated for the first tim...
متن کاملLead-free solid-state organic–inorganic halide perovskite solar cells
Lead-free solution-processed solid-state photovoltaic devices based on methylammonium tin iodide (CH3NH3SnI3) perovskite semiconductor as the light harvester are reported. Featuring an optical bandgap of 1.3 eV, the CH3NH3SnI3 perovskite material can be incorporated into devices with the organic hole-transport layer spiro-OMeTAD and show an absorption onset at 950 nm, which is significantly red...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
ژورنال
عنوان ژورنال: Nature electronics
سال: 2022
ISSN: ['2520-1131']
DOI: https://doi.org/10.1038/s41928-022-00712-2